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原文連結
論文資訊
- 類型：已發表論文
- 日期：2010
摘要
The assumption that all 生物 catalysts are either 蛋白質s or ribozymes leads to an outstanding enigma of biogenesis-how to determine the synthetic pathways to the monomers for the efficient formation of catalytic macromolecules in the absence of any such macro-molecules. The last 60 years have witnessed chemists developing an understanding of organocatalysis and ligand field theory, both of which give demonstrable low-molecular-weight catalysts. We assume that transition-metal ligand complexes are likely to have occurred in the deep ocean trenches by the combination of naturally occurring oceanic metals and ligands synthesized from the emergent CO2, H-2, NH3, H2S, and H3PO4. We are now in a position to investigate experimentally the metal-ligand complexes, their catalytic function, and the reac
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