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原文連結
論文資訊
- 類型:已發表論文
- 日期:2014-06-23
摘要
Starting from our recent chemical master equation derivation of the model of an autocatalytic reaction-擴散 chemical system with reactions U + 2V<(lambda(0))under right arrow>3V and V<(mu)under right arrow>P, U<(nu)under right arrow>Q, we determine the effects of intrinsic noise on the momentum-space behavior of its kinetic parameters and chemical concentrations. We demonstrate that the intrinsic noise induces n -> n molecular interaction processes with n >= 4, where n is the number of participating molecules of type U or V. The momentum dependences of the reaction rates are driven by the fact that the autocatalytic reaction (inelastic scattering) is renormalized through the existence of an arbitrary number of intermediate elastic scatterings, which can also be interpreted as the creation an
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