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論文資訊
- 類型:已發表論文
- 日期:2021-08-20
摘要
The design and chemical synthesis of artificial material objects which can mimic the functions of living cells is an important ongoing scientific endeavor. A key challenge necessary for fulfilling the criteria for a system to be living currently regards 演化, which is derived from adaptivity. Integrated chemical loops capable of feedback control are required to achieve chemical systems which exhibit adaptivity. To explore this, we present an integrated, two-component orthogonal chemical process involving reversible addition–fragmentation chain transfer (RAFT) based polymerization-induced self-assembly (PISA) and a copper-catalyzed azide–alkyne click (CuAAC) coupling reaction. The chemical processes are linked through electron transfer from the activated chain-transfer 智能體 (CTA) to the dorman
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